Precursor-Dependent Performance of FA-, GBFS-, MK- and WBP-Based Geopolymer Mortars: Effects of NaOH Molarity and Thermal Curing on Strength, Transport Properties and Cost Efficiency


ÇELİK D. N., Demircan R. K., Avinç G. M., KAPLAN G.

Polymers, cilt.18, sa.14, 2026 (SCI-Expanded, Scopus)

  • Yayın Türü: Makale / Tam Makale
  • Cilt numarası: 18 Sayı: 14
  • Basım Tarihi: 2026
  • Doi Numarası: 10.3390/polym18141723
  • Dergi Adı: Polymers
  • Derginin Tarandığı İndeksler: Science Citation Index Expanded (SCI-EXPANDED), Scopus, Chemical Abstracts Core, Compendex, INSPEC, Academic Search Ultimate (EBSCO), Engineering Source (EBSCO), Materials Science & Engineering Collection (ProQuest), Technology Collection (ProQuest)
  • Anahtar Kelimeler: alkali activation, chloride-ion penetration, cost index, electrical resistivity, waste brick powder
  • Atatürk Üniversitesi Adresli: Evet

Özet

This study investigated the effects of precursor type, NaOH molarity, and thermal curing temperature on the performance of geopolymer mortars produced using fly ash (FA), ground granulated blast-furnace slag (GBFS), metakaolin (MK), and waste brick powder (WBP). Mortars were activated using 12 M and 16 M NaOH solutions at a constant Na2SiO3/NaOH ratio and thermally cured at 60 and 90 °C for 24 h. Physical, mechanical, transport, microstructural, and cost-performance properties were evaluated. The results demonstrated that the optimum activation conditions strongly depended on precursor type. MK-based mortars cured at 16 M–90 °C exhibited the best overall performance, achieving the lowest apparent porosity (6.1%) and water absorption (5.4%), and the highest oven-dry density (2194 kg/m3), compressive strength (25.8 MPa), and flexural strength (3.43 MPa). These mortars also exhibited the lowest capillary water absorption (1.88 kg/m2), the highest electrical resistivity (248.00 kΩ·cm), and the lowest charge passed (177 C), indicating enhanced pore refinement and chloride-ion penetrability. In contrast, GBFS performed better under milder activation conditions, whereas WBP showed lower performance due to its coarser, more crystalline structure. SEM/EDS analyses confirmed that the formation of dense aluminosilicate gel governed matrix quality and overall performance. Overall, MK activated at 16 M and cured at 90 °C provided the most favorable balance between technical performance and cost efficiency.